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Creators/Authors contains: "Yang, Ming"

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  1. Free, publicly-accessible full text available September 1, 2024
  2. Free, publicly-accessible full text available July 1, 2024
  3. Abstract

    Copper-based catalyst is uniquely positioned to catalyze the hydrocarbon formations through electrochemical CO2reduction. The catalyst design freedom is limited for alloying copper with H-affinitive elements represented by platinum group metals because the latter would easily drive the hydrogen evolution reaction to override CO2reduction. We report an adept design of anchoring atomically dispersed platinum group metal species on both polycrystalline and shape-controlled Cu catalysts, which now promote targeted CO2reduction reaction while frustrating the undesired hydrogen evolution reaction. Notably, alloys with similar metal formulations but comprising small platinum or palladium clusters would fail this objective. With an appreciable amount of CO-Pd1moieties on copper surfaces, facile CO*hydrogenation to CHO*or CO-CHO*coupling is now viable as one of the main pathways on Cu(111) or Cu(100) to selectively produce CH4or C2H4through Pd-Cu dual-site pathways. The work broadens copper alloying choices for CO2reduction in aqueous phases.

     
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  4. Abstract

    Referring expression comprehension aims to localize objects identified by natural language descriptions. This is a challenging task as it requires understanding of both visual and language domains. One nature is that each object can be described by synonymous sentences with paraphrases, and such varieties in languages have critical impact on learning a comprehension model. While prior work usually treats each sentence and attends it to an object separately, we focus on learning a referring expression comprehension model that considers the property in synonymous sentences. To this end, we develop an end-to-end trainable framework to learn contrastive features on the image and object instance levels, where features extracted from synonymous sentences to describe the same object should be closer to each other after mapping to the visual domain. We conduct extensive experiments to evaluate the proposed algorithm on several benchmark datasets, and demonstrate that our method performs favorably against the state-of-the-art approaches. Furthermore, since the varieties in expressions become larger across datasets when they describe objects in different ways, we present the cross-dataset and transfer learning settings to validate the ability of our learned transferable features.

     
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